In-situ X-ray studies of clean catalytic technologies

Adam F. Lee; Christine V. Ellis; Mark A Newton; Christopher M. Parlett; Karen Wilson

doi:10.1557/opl.2011.1170

In-situ X-ray studies of clean catalytic technologies

Adam F. Lee, Christine V. Ellis, Mark A Newton, Christopher M. Parlett, Karen Wilson

Research output: Chapter in Book/Published conference output › Conference publication

Abstract

The rational design of new heterogeneous catalysts for clean chemical technologies can be accelerated by molecular level insight into surface chemical processes. In-situ methodologies, able to provide time-resolved and/or pressure dependent information on the evolution of reacting adsorbed layers over catalytically relevant surfaces, are therefore of especial interest. Here we discuss the application of in-situ XPS and in-situ, synchronous DRIFTS/MS/XAS methodologies to elucidate the active site in Pd-catalyzed, selective aerobic oxidation of allylic alcohols.

Original language	English
Title of host publication	2011 MRS spring meeting
Subtitle of host publication	symposium FF : surfaces and nanomaterials for catalysis through in-situ or ex-situ studies
Editors	F. Tao, M. Salmeron, J.A. Rodriguez, J. Hu
Place of Publication	Cambridge (UK)
Publisher	Cambridge University Press
ISBN (Print)	978-1-6183-9554-2
DOIs	https://doi.org/10.1557/opl.2011.1170
Publication status	Published - 2011
Event	2011 MRS Spring Meeting & Exhibit - San Francisco, CA, United States Duration: 25 Apr 2011 → 29 Apr 2011

Publication series

Name	MRS proceedings
Volume	1351

Conference

Conference	2011 MRS Spring Meeting & Exhibit
Country/Territory	United States
City	San Francisco, CA
Period	25/04/11 → 29/04/11

Keywords

Pd
oxidation
extended x-ray absorption fine structure

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10.1557/opl.2011.1170

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Lee, A. F., Ellis, C. V., Newton, M. A., Parlett, C. M., & Wilson, K. (2011). In-situ X-ray studies of clean catalytic technologies. In F. Tao, M. Salmeron, J. A. Rodriguez, & J. Hu (Eds.), 2011 MRS spring meeting: symposium FF : surfaces and nanomaterials for catalysis through in-situ or ex-situ studies Article mrss11-1351-ff16-05 (MRS proceedings; Vol. 1351). Cambridge University Press. https://doi.org/10.1557/opl.2011.1170

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title = "In-situ X-ray studies of clean catalytic technologies",

abstract = "The rational design of new heterogeneous catalysts for clean chemical technologies can be accelerated by molecular level insight into surface chemical processes. In-situ methodologies, able to provide time-resolved and/or pressure dependent information on the evolution of reacting adsorbed layers over catalytically relevant surfaces, are therefore of especial interest. Here we discuss the application of in-situ XPS and in-situ, synchronous DRIFTS/MS/XAS methodologies to elucidate the active site in Pd-catalyzed, selective aerobic oxidation of allylic alcohols.",

keywords = "Pd, oxidation, extended x-ray absorption fine structure",

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language = "English",

isbn = "978-1-6183-9554-2",

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editor = "F. Tao and M. Salmeron and J.A. Rodriguez and J. Hu",

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Lee, AF, Ellis, CV, Newton, MA, Parlett, CM & Wilson, K 2011, In-situ X-ray studies of clean catalytic technologies. in F Tao, M Salmeron, JA Rodriguez & J Hu (eds), 2011 MRS spring meeting: symposium FF : surfaces and nanomaterials for catalysis through in-situ or ex-situ studies., mrss11-1351-ff16-05, MRS proceedings, vol. 1351, Cambridge University Press, Cambridge (UK), 2011 MRS Spring Meeting & Exhibit, San Francisco, CA, United States, 25/04/11. https://doi.org/10.1557/opl.2011.1170

In-situ X-ray studies of clean catalytic technologies. / Lee, Adam F.; Ellis, Christine V.; Newton, Mark A et al.
2011 MRS spring meeting: symposium FF : surfaces and nanomaterials for catalysis through in-situ or ex-situ studies. ed. / F. Tao; M. Salmeron; J.A. Rodriguez; J. Hu. Cambridge (UK): Cambridge University Press, 2011. mrss11-1351-ff16-05 (MRS proceedings; Vol. 1351).

Research output: Chapter in Book/Published conference output › Conference publication

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N2 - The rational design of new heterogeneous catalysts for clean chemical technologies can be accelerated by molecular level insight into surface chemical processes. In-situ methodologies, able to provide time-resolved and/or pressure dependent information on the evolution of reacting adsorbed layers over catalytically relevant surfaces, are therefore of especial interest. Here we discuss the application of in-situ XPS and in-situ, synchronous DRIFTS/MS/XAS methodologies to elucidate the active site in Pd-catalyzed, selective aerobic oxidation of allylic alcohols.

AB - The rational design of new heterogeneous catalysts for clean chemical technologies can be accelerated by molecular level insight into surface chemical processes. In-situ methodologies, able to provide time-resolved and/or pressure dependent information on the evolution of reacting adsorbed layers over catalytically relevant surfaces, are therefore of especial interest. Here we discuss the application of in-situ XPS and in-situ, synchronous DRIFTS/MS/XAS methodologies to elucidate the active site in Pd-catalyzed, selective aerobic oxidation of allylic alcohols.

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Lee AF, Ellis CV, Newton MA, Parlett CM, Wilson K. In-situ X-ray studies of clean catalytic technologies. In Tao F, Salmeron M, Rodriguez JA, Hu J, editors, 2011 MRS spring meeting: symposium FF : surfaces and nanomaterials for catalysis through in-situ or ex-situ studies. Cambridge (UK): Cambridge University Press. 2011. mrss11-1351-ff16-05. (MRS proceedings). doi: 10.1557/opl.2011.1170

In-situ X-ray studies of clean catalytic technologies

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