Tailored mesoporous silica supports for Ni catalysed hydrogen production from ethanol steam reforming

Christopher M.A. Parlett; Ayse Aydin; Lee J. Durndell; Lucia Frattini; Mark A. Isaacs; Adam F. Lee; Xiaotong Liu; Luca Olivi; Rima Trofimovaite; Karen Wilson; Chunfei Wu

doi:10.1016/j.catcom.2016.12.021

Tailored mesoporous silica supports for Ni catalysed hydrogen production from ethanol steam reforming

Christopher M.A. Parlett^*
, Ayse Aydin
, Lee J. Durndell
, Lucia Frattini
, Mark A. Isaacs
, Adam F. Lee
, Xiaotong Liu
, Luca Olivi
, Rima Trofimovaite
, Karen Wilson
, Chunfei Wu

^*Corresponding author for this work

University of Hull
Sincrotrone Trieste

Research output: Contribution to journal › Article › peer-review

58 Citations (Scopus)

184 Downloads (Pure)

Abstract

Mesoporous silica supported Ni nanoparticles have been investigated for hydrogen production from ethanol steam reforming. Ethanol reforming is structure-sensitive over Ni, and also dependent on support mesostructure; three-dimensional KIT-6 possessing interconnected mesopores offers superior metal dispersion, steam reforming activity, and on-stream stability against deactivation compared with a two-dimensional SBA-15 support.

Original language	English
Pages (from-to)	76-79
Number of pages	4
Journal	Catalysis Communications
Volume	91
Early online date	21 Dec 2016
DOIs	https://doi.org/10.1016/j.catcom.2016.12.021
Publication status	Published - 5 Mar 2017

Bibliographical note

© 2016, Elsevier. Licensed under the Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International http://creativecommons.org/licenses/by-nc-nd/4.0/

Funding: EPSRC (EP/N009924/1); Sincrotrone Trieste for the award of XAS beamtime (20155166); and Erasmus Internship Program.

Supplementary data available on the journal website.

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

SDG 7 Affordable and Clean Energy

Keywords

ethanol steam reforming
hydrogen production
mesoporous materials
nanoparticles
nickel

Access to Document

10.1016/j.catcom.2016.12.021

Ni catalysed hydrogen production from ethanol steam reforming
© 2016, Elsevier. Licensed under the Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International http://creativecommons.org/licenses/by-nc-nd/4.0/
Accepted author manuscript, 684 KBLicence: CC BY-NC-ND 3.0

Cite this

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title = "Tailored mesoporous silica supports for Ni catalysed hydrogen production from ethanol steam reforming",

abstract = "Mesoporous silica supported Ni nanoparticles have been investigated for hydrogen production from ethanol steam reforming. Ethanol reforming is structure-sensitive over Ni, and also dependent on support mesostructure; three-dimensional KIT-6 possessing interconnected mesopores offers superior metal dispersion, steam reforming activity, and on-stream stability against deactivation compared with a two-dimensional SBA-15 support.",

keywords = "ethanol steam reforming, hydrogen production, mesoporous materials, nanoparticles, nickel",

author = "Parlett, \{Christopher M.A.\} and Ayse Aydin and Durndell, \{Lee J.\} and Lucia Frattini and Isaacs, \{Mark A.\} and Lee, \{Adam F.\} and Xiaotong Liu and Luca Olivi and Rima Trofimovaite and Karen Wilson and Chunfei Wu",

note = "{\textcopyright} 2016, Elsevier. Licensed under the Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International http://creativecommons.org/licenses/by-nc-nd/4.0/ Funding: EPSRC (EP/N009924/1); Sincrotrone Trieste for the award of XAS beamtime (20155166); and Erasmus Internship Program. Supplementary data available on the journal website.",

year = "2017",

month = mar,

day = "5",

doi = "10.1016/j.catcom.2016.12.021",

language = "English",

volume = "91",

pages = "76--79",

journal = "Catalysis Communications",

issn = "1566-7367",

publisher = "Elsevier",

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TY - JOUR

T1 - Tailored mesoporous silica supports for Ni catalysed hydrogen production from ethanol steam reforming

AU - Parlett, Christopher M.A.

AU - Aydin, Ayse

AU - Durndell, Lee J.

AU - Frattini, Lucia

AU - Isaacs, Mark A.

AU - Lee, Adam F.

AU - Liu, Xiaotong

AU - Olivi, Luca

AU - Trofimovaite, Rima

AU - Wilson, Karen

AU - Wu, Chunfei

N1 - © 2016, Elsevier. Licensed under the Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International http://creativecommons.org/licenses/by-nc-nd/4.0/ Funding: EPSRC (EP/N009924/1); Sincrotrone Trieste for the award of XAS beamtime (20155166); and Erasmus Internship Program. Supplementary data available on the journal website.

PY - 2017/3/5

Y1 - 2017/3/5

N2 - Mesoporous silica supported Ni nanoparticles have been investigated for hydrogen production from ethanol steam reforming. Ethanol reforming is structure-sensitive over Ni, and also dependent on support mesostructure; three-dimensional KIT-6 possessing interconnected mesopores offers superior metal dispersion, steam reforming activity, and on-stream stability against deactivation compared with a two-dimensional SBA-15 support.

AB - Mesoporous silica supported Ni nanoparticles have been investigated for hydrogen production from ethanol steam reforming. Ethanol reforming is structure-sensitive over Ni, and also dependent on support mesostructure; three-dimensional KIT-6 possessing interconnected mesopores offers superior metal dispersion, steam reforming activity, and on-stream stability against deactivation compared with a two-dimensional SBA-15 support.

KW - ethanol steam reforming

KW - hydrogen production

KW - mesoporous materials

KW - nanoparticles

KW - nickel

UR - http://doi.org/10.17036/researchdata.aston.ac.uk.00000186

UR - https://www.scopus.com/pages/publications/85007565840

U2 - 10.1016/j.catcom.2016.12.021

DO - 10.1016/j.catcom.2016.12.021

M3 - Article

SN - 1566-7367

VL - 91

SP - 76

EP - 79

JO - Catalysis Communications

JF - Catalysis Communications

ER -

Tailored mesoporous silica supports for Ni catalysed hydrogen production from ethanol steam reforming

Abstract

Bibliographical note

UN SDGs

Keywords

Access to Document

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