We observe strongly dissimilar scattering from two types of edges in hexagonal quasi-monocrystalline gold flakes with thicknesses around 1 micron. We identify as the origin the interference between a direct, quasi-specular scattering and an indirect scattering process involving an intermediate surface-plasmon state. The dissimilarity between the two types of edges is a direct consequence of the three-fold symmetry around the -axis and the intrinsic chirality of a face-centered cubic lattice. We propose that this effect can be used to estimate flake thickness, crystal morphology, and surface contamination.
|Publication status||Published - 5 Sep 2018|
Bibliographical note© 2018 The Authors.
Funding: MSCA-COFUND-MULTIPLY - Grant number 713694 - H2020.
Boroviks, S., Wolff, C., Linnet, J., Yang, Y., Todisco, F., Roberts, A. S., Bozhevolnyi, S. I., Hecht, B., & Mortensen, N. A. (2018). Interference in edge-scattering from monocrystalline gold flakes. https://arxiv.org/abs/1809.01542